Characterization of the sulphate mineral amarantite - using infrared, Raman spectroscopy and thermogravimetry.

Abstract
The mineral amarantite Fe3þ 2 (SO4)O _ 7H2O has been studied using a combination of techniques including thermogravimetry, electron probe analyses and vibrational spectroscopy. Thermal analysis shows decomposition steps at 77.63, 192.2, 550 and 641.4 _C. The Raman spectrum of amarantite is dominated by an intense band at 1017 cm_1 assigned to the SO2_ 4 m1 symmetric stretching mode. Raman bands at 1039, 1054, 1098, 1131, 1195 and 1233 cm_1 are attributed to the SO2_ 4 m3 antisymmetric stretching modes. Very intense Raman band is observed at 409 cm_1 with shoulder bands at 399, 451 and 491 cm_1 are assigned to the m2 bending modes. A series of low intensity Raman bands are found at 543, 602, 622 and 650 cm_1 are assigned to the m4 bending modes. A very sharp Raman band at 3529 cm_1 is assigned to the stretching vibration of OH units. A series of Raman bands observed at 3025, 3089, 3227, 3340, 3401 and 3480 cm_1 are assigned to water bands. Vibrational spectroscopy enables aspects of the molecular structure of the mineral amarantite to be ascertained.
Description
Keywords
Raman spectroscopy, Amarantite, Infrared spectroscopy, Sulphate, Evaporite
Citation
FROST, R. L. et al. Characterization of the sulphate mineral amarantite - using infrared, Raman spectroscopy and thermogravimetry. Disponível em: <http://www.sciencedirect.com/science/article/pii/S1386142513004605>. Acesso em: 07 out. 2014.
https://doi.org/10.1016/j.saa.2013.04.111